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Unknot

ʌnˈnɒt

Unknot definitions
verb
unknots unknotting unknotted unknot
  1. release or untie the knot or knots in

    "he swiftly unknotted his tie"

  2. (of a muscle) relax after being tense and hard

    "his shoulders unknotted"

    become less tense become less stiff/rigid loosen slacken ease unknot